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The effect of adding 0-10% w/w of carboxymethylcellulose (CMC) to the alginate solutions was studied, as well as the effect of incorporating 0-50% w/w of alginate and chitosan into the CMC/alginate composite. The degree of pore interconnectivity and permeability was determined using mercury intrusion porosimetry and osmotic pressure measurements. Porogen type and inclusion of the alginate/chitosan components significantly affected the mechanical properties of the scaffolds, with the most porous composite scaffolds being the weakest. Porosity, permeability and specific surface area of the samples were dependent on the porogen type used. The pore interconnectivity of the composite scaffolds was highest for cmAA and least for amAA. Elastic modulus, yield stress and ultimate strength were also significantly affected by the porogen type, composite ratio, and processing method. 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